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1.核科学与工程学院 华北电力大学 北京 102206
2.国家核安保技术中心 北京 102401
3.中广核研究院有限公司 深圳 518031
4.深圳市核与辐射安全重点实验室,中国核能与安全高等研究院, 深圳大学 物理与光电工程学院 深圳 518060
刘月壮,男,1994年出生,2021年于华北电力大学获硕士学位,研究领域为核材料衡算
张小东,E-mail:zhangxiaodong@szu.edu.cn
收稿日期:2024-09-14,
修回日期:2025-01-12,
网络出版日期:2025-03-31,
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刘月壮, 张少东, 尤园江, 等. 基于液体闪烁体探测器的被动法快中子多重性测量装置的研制[J/OL]. 核技术, 2025,XXXXXX
LIU Yuezhuang, ZHANG Shaodong, YOU Yuanjiang, et al. R&D of passive fast neutron multiplicity counting system based on liquid scintillation detectors[J/OL]. Nuclear techniques, 2025, XXXXXX
刘月壮, 张少东, 尤园江, 等. 基于液体闪烁体探测器的被动法快中子多重性测量装置的研制[J/OL]. 核技术, 2025,XXXXXX DOI: 10.11889/j.0253-3219.2025.hjs.48.240364. CSTR: 32193.14.hjs.CN31-1342/TL.2025.48.240364.
LIU Yuezhuang, ZHANG Shaodong, YOU Yuanjiang, et al. R&D of passive fast neutron multiplicity counting system based on liquid scintillation detectors[J/OL]. Nuclear techniques, 2025, XXXXXX DOI: 10.11889/j.0253-3219.2025.hjs.48.240364. CSTR: 32193.14.hjs.CN31-1342/TL.2025.48.240364.
快中子多重性测量技术能够快速、准确地检测出特殊核材料(Special Nuclear Materials,SNM)中
240
Pu的有效质量,对防止核扩散具有重要意义。本文详细介绍了团队开发的一套被动快中子多重性测量装置,该装置主要由32个自主研发的EJ-309液体闪烁探测器组成。为提高探测效率的均匀性,这些探测器以球对称形式排布。此外,该装置集成了自主设计开
发的32通道的高压电源以及用户友好图形界面。数据分析采用双重(Doubles)参数拟合和快中子多重性分析两种方法。对该装置的测试结果表明:该装置能够准确计算出
252
Cf中子源(等效
240
Pu有效质量为5.37~209.62 g)的自发裂变率。此外,该装置还在不同的环境本底(总中子计数率Singles分别为111.42±0.46、73.97±0.28、47.27±0.29)下进行测试。测量结果与低本底下(Singles计数率为0.51±0.02)的测量结果基本一致,这表明该装置具有非常好的抗本底干扰能力。
Background
2
Traditional thermal/epithermal neutron multiplicity counting systems based on
3
He tubes have relatively low measurement accuracy and high development costs. Fast neutron multiplicity counting (FNMC) technique based on liquid scintillation detectors has become a research hotspot. However
fast neutron multiplicity counting systems currently built are still in the experimental research stage.
Purpose
2
This study aims to develop a passive fast neutron multiplicity counting system that can be used for practical measurement.
Method
2
Firstly
a passive fast neutron multiplicity counting system was built using 32 self-developed EJ-309 liquid scintillation detectors. To improve the uniformity of neutron detection efficiency of the system
these detectors were arranged in a spherically symmetrical geometry. The system also integrated a self-designed and developed 32-channel high-voltage power supply and a user-friendly graphical interface. Secondly
the Doubles parameter fitting method and the three-parameter fast neutron multiplicity analytical method were used to evaluate the spontaneous fission rates of the
252
Cf neutron sources respectively. Finally
the performance of the system under different neutron radiation backgrounds (with Singles rates of 111.42±0.46
73.97±0.28
and 47.27±0.29
respectively) was also evaluated.
Results
2
The experimental results show that the Doubles parameter fitting method can accurately evaluate the spontaneous fission rates of
252
Cf neutron sources. The relative differences of the spontaneous f
ission rates of the
252
Cf neutron sources evaluated by using the fast neutron multiplicity analytical method are less than ±4%. The measurement results under different neutron radiation backgrounds are basically consistent with those under natural environment background (the Singles rates were 0.51±0.02).
Conclusions
2
The FNMC system can accurately determine the spontaneous fission rate of the
252
Cf neutron source (with an equivalent
240
Pu
eff
mass range of 5.37~209.62 g)
and has very good anti-background interference capabilities.
Balatsky G I , Severe W R . Illicit trafficking of radioactive and nuclear materials [M ] . Nuclear Safeguards, Security, and Nonproliferation . Amsterdam : Elsevier , 2019 : 357 – 387 . DOI: 10.1016/b978-0-12-803271-8.00012-6 http://dx.doi.org/10.1016/b978-0-12-803271-8.00012-6 .
Böhnel K . The effect of multiplication on the quantitative determination of spontaneously fissioning isotopes by neutron correlation analysis [J ] . Nuclear Science and Engineering , 1985 , 90 ( 1 ): 75 – 82 . DOI: 10.13182/NSE85-2 http://dx.doi.org/10.13182/NSE85-2 .
Langner D , Stewart J , Pickrell M , et al . Application guide to neutron multiplicity counting [R ] . Los Alamos : Los Alamos National Laboratory , 1999 . 10.2172/1679 http://dx.doi.org/10.2172/1679
Chichester D , Pozzi S , Dolan J , et al . MPACT fast neutron multiplicity system prototype development [R ] . Idaho Falls : Idaho National Laboratory (INL) , 2013 . 10.2172/1111016 http://dx.doi.org/10.2172/1111016
Lavietes A , Plenteda R , Mascarenhas N , et al . Liquid scintillator-based neutron detector development [C ] . 2012 IEEE Nuclear Science Symposium and Medical Imaging Conference Record (NSS/MIC). October 27 - November 3 , 2012 , Anaheim, CA, USA. IEEE , 2012: 230 – 244 . DOI: 10.1109/NSSMIC.2012.6551100 http://dx.doi.org/10.1109/NSSMIC.2012.6551100 .
Joyce M J , Gamage K A A , Aspinall M D , et al . A 4-channel multiplex analyzer for real-time, parallel processing of fast scintillators [C ] . 2012 IEEE Nuclear Science Symposium and Medical Imaging Conference Record (NSS/MIC). October 27 - November 3 , 2012 , Anaheim, CA, USA. IEEE , 2012: 134 – 138 . DOI: 10.1109/NSSMIC.2012.6551077 http://dx.doi.org/10.1109/NSSMIC.2012.6551077 .
Wachter J R , Adams E L , Ensslin N . Prototype fast neutron counter for the assay of impure plutonium [R ] . Los Alamos National Laboratory (LANL), Los Alamos, NM (United States) , 1987 .
Shin T . Fast-neutron multiplicity counting techniques for nuclear safeguards applications [D ] . Ann Arbor : University of Michigan , 2019 . 10.1109/nssmic.2018.8824630 http://dx.doi.org/10.1109/nssmic.2018.8824630
Di Fulvio A , Shin T H , Jordan T , et al . Passive assay of plutonium metal plates using a fast-neutron multiplicity counter [J ] . Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment , 2017 , 855 : 92 – 101 . DOI: 10.1016/j.nima.2017.02.082 http://dx.doi.org/10.1016/j.nima.2017.02.082 .
Shin T H , Hua M Y , Marcath M J , et al . Neutron multiplicity counting moments for fissile mass estimation in scatter-based neutron detection systems [J ] . Nuclear Science and Engineering , 2017 , 188 ( 3 ): 246 – 269 . DOI: 10.1080/00295639.2017.1354591 http://dx.doi.org/10.1080/00295639.2017.1354591 .
Sarwar R , Astromskas V , Zimmerman C H , et al . An event-triggered coincidence algorithm for fast-neutron multiplicity assay corrected for cross-talk and photon breakthrough [J ] . Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment , 2018 , 903 : 152 – 161 . DOI: 10.1016/j.nima.2018.06.056 http://dx.doi.org/10.1016/j.nima.2018.06.056 .
Joyce M J , Sarwar R , Astromskas V , et al . High-order angular correlation of californium-252 fission neutrons and the effect of detector cross-talk [J ] . Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment , 2020 , 954 : 161866 . DOI: 10.1016/j.nima. 2019.01.092 http://dx.doi.org/10.1016/j.nima.2019.01.092 .
Zhang Q H , Li S F , Zhuang L , et al . Simulation study on neutron multiplicity of plutonium based on liquid scintillation detector [J ] . Applied Radiation and Isotopes , 2018 , 135 : 92 – 98 . DOI: 10.1016/j.apradiso.2018.01.022 http://dx.doi.org/10.1016/j.apradiso.2018.01.022 .
Li S F , Qiu S Z , Zhang Q H , et al . Fast-neutron multiplicity analysis based on liquid scintillation [J ] . Applied Radiation and Isotopes , 2016 , 110 : 53 – 58 . DOI: 10.1016/j.apradiso.2015.12.064 http://dx.doi.org/10.1016/j.apradiso.2015.12.064 .
Zhang Q H , Su X H , Hou S X , et al . Analysis and improvement of the influence of sample shape on Pu measurement results [J ] . Journal of Nuclear Science and Technology , 2020 , 57 ( 6 ): 678 – 688 . DOI: 10.1080/00223131.2020.1715898 http://dx.doi.org/10.1080/00223131.2020.1715898 .
程毅梅 , 许小明 , 尹洪河 , 等 . 用于核保障中核材料衡算的液体闪烁体中子多重性测量装置 [J ] . 原子能科学技术 , 2020 , 54 ( 6 ): 1132 – 1139 . DOI: 10.7538/yzk.2019.youxian.0318 http://dx.doi.org/10.7538/yzk.2019.youxian.0318 .
CHENG Yimei , XU Xiaoming , YIN Honghe , et al . Liquid scintillation detector based neutron multiplicity counting device for nuclear material accountancy in nuclear safeguard [J ] . Atomic Energy Science and Technology , 2020 , 54 ( 6 ): 1132 – 1139 . DOI: 10.7538/yzk.2019.youxian.0318 http://dx.doi.org/10.7538/yzk.2019.youxian.0318 .
张小东 , 刘月壮 , 张琦 , 等 . 一种基于球对称结构的被动核材料快中子多重性测量系统 : CN216669794U [P ] . 2022-06-03 .
ZHANG Xiaodong , LIU Yuezhuang , ZHANG Qi , et al . A fast neutron multiplicity measurement system for passive nuclear materials based on spherically symmetric structure : CN216669794U [P ] . 2022-06-03 .
CAEN , User manual UM 4279 V 1742 B[EB/OL ] . ( 2022-04-04 ) [ 2023-06-21 ] . https://www.caen.it/products/V1742/ https://www.caen.it/products/V1742/ .
Croft S , Cleveland S L , Nicholson A D . Calculation of the 240 Pu-Effective coefficients for neutron correlation counting-INMM [R ] . Oak Ridge : Oak Ridge National Laboratory , 2015 .
Moszyński M , Costa G J , Guillaume G , et al . Study of n-γ discrimination with NE213 and BC501A liquid scintillators of different size [J ] . Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment , 1994 , 350 ( 1–2 ): 226 – 234 . DOI: 10.1016/0168-9002(94)91169-X http://dx.doi.org/10.1016/0168-9002(94)91169-X .
张少东 , 金宝亮 , 张小东 . 基于液闪EJ301研制的中子探测器的性能测试 [J ] . 核技术 , 2024 , 47 ( 8 ): 080402 . DOI: 10.11889/j.0253-3219.2024.hjs.47.080402 http://dx.doi.org/10.11889/j.0253-3219.2024.hjs.47.080402 .
ZHANG Shaodong , JIN Baoliang , ZHANG Xiaodong . Evaluation of self-developed neutron detector based on EJ301 liquid scintillator [J ] . Nuclear Techniques , 2024 , 47 ( 8 ): 080402 . DOI: 10.11889/j.0253-3219.2024.hjs.47.080402 http://dx.doi.org/10.11889/j.0253-3219.2024.hjs.47.080402 .
常乐 , 刘应都 , 杜龙 , 等 . EJ301液体闪烁体探测器的波形甄别和能量刻度 [J ] . 核技术 , 2015 , 38 ( 2 ): 020501 . DOI: 10.11889/j.0253-3219.2015.hjs.38.020501 http://dx.doi.org/10.11889/j.0253-3219.2015.hjs.38.020501 .
CHANG Le , LIU Yingdu , DU Long , et al . Pulse shape discrimination and energy calibration of EJ301 liquid scintillation detector [J ] . Nuclear Techniques , 2015 , 38 ( 2 ): 020501 . DOI: 10.11889/j.0253-3219.2015.hjs.38.020501 http://dx.doi.org/10.11889/j.0253-3219.2015.hjs.38.020501 .
Liu M Z , Liu B Q , Zuo Z , et al . Toward a fractal spectrum approach for neutron and gamma pulse shape discrimination [J ] . Chinese Physics C , 2016 , 40 ( 6 ): 066201 . DOI: 10.1088/1674-1137/40/6/066201 http://dx.doi.org/10.1088/1674-1137/40/6/066201 .
Valentine T . Preliminary evaluation of NMIS for interrogation of Pu and HEU in AT400-RContainers at mayak [R ] . Oak Ridge : Oak Ridge National Laboratory , 2000 . 10.2172/885755 http://dx.doi.org/10.2172/885755
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