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1. 南华大学 核科学技术学院 氡湖南省重点实验室,衡阳,421001
2. 中国科学院上海应用物理研究所 嘉定园区,上海,201800
[ "通讯作者: 刘晓翔 E-mail:shine6@foxmail.com" ]
纸质出版日期:2015-11-13
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单 健, 刘晓翔, 肖德涛, 等. 大气颗粒物中210Pb的活度-粒径分布测量[J]. 核技术, 2015,38(11):110303
SHAN Jian, LIU Xiaoxiang, XIAO Detao, et al. Measurement of the activity-size distribution of 210Pb in atmospheric particulates[J]. Nuclear techniques, 2015, 38(11): 110303
单 健, 刘晓翔, 肖德涛, 等. 大气颗粒物中210Pb的活度-粒径分布测量[J]. 核技术, 2015,38(11):110303 DOI: 10.11889/j.0253-3219.2015.hjs.38.110303.
SHAN Jian, LIU Xiaoxiang, XIAO Detao, et al. Measurement of the activity-size distribution of 210Pb in atmospheric particulates[J]. Nuclear techniques, 2015, 38(11): 110303 DOI: 10.11889/j.0253-3219.2015.hjs.38.110303.
用M235大气颗粒物分级采样器采样获得不同范围粒径的可吸入大气颗粒物样品,然后分别用?分析方法和?分析方法测量不同粒径尺度样品中的210Pb的活度分布。得到大气颗粒物样品中210Pb的体积比活度在不同粒径上的分布范围为0.004 4–1.832 1mBq·m?3,最大值均落在0.49–0.95?m粒径范围。两种分析方法所测得的数据具有近似的活度-粒径分布关系,其离散性变化规律也基本一致,都是在粒径范围为0.49–1.5?m之间的标准差最大,?计数法测量的数据离散性整体比?计数法测量的数据偏大。
Background: 210Pb in air has yielded insight on the sources and transit times of aerosols. In an ideal enclosed air mass (closed system with respect to these nuclides)
the residence times of aerosols can be obtained from the activity ratios of 210Pb/222Rn
210Bi/210Pb
and 210Po/210Pb. Through measuring the activity-size distribution of 210Pb in the atmospheric particulates
it is conducive to the use of 210Pb tracer study in atmosphere. Purpose: This study aims to determine the activity-size distribution of 210Pb in the atmospheric particulates. Methods: Inhalable particles samples at different particle size levels were collected by M235 impact large flow classification sampler. The activity distribution of 210Pb in different particle size scales was determined by detecting β rays of 210Bi (the first generation progeny of 210Pb)
and radioactivity of 210Pb was determined by using γ spectrometer
respectively. Results: Experimental results show that the distribution range of the specific activity (mBq·m?3) of 210Pb in atmospheric particulates is 0.0044–1.8321mBq·m?3 and the maximum are within 0.49–0.95μm size distribution. Conclusion: The activity-size distribution of 210Pb in the atmospheric particulates is mainly due to the effects of temperature
humidity
rainfall
wind speed
wind direction and other natural factors; the discrete of β counting measured data is larger than the discrete of γ counting measured data. Abstract
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